Method for Deriving the Complex Infrared Dielectric Function of Amorphous Thin Films from Infrared Reflectivity Spectroscopy
Marwa Youssef Dakik, Michel Kazan
كلية العلوم والأداب-الجامعة الأمريكية في بيروت · لبنان
الموضوعات
علوم بحتة وطبيعية
الملخص
Although advanced nonlinear optical techniques have demonstrated high potentialfor examining elementary excitations in semiconductors, infrared reflectivityanalysis remains the most quantitative technique because simple theories canbe used to describe the material response to an infrared wavelength excitation.Line shape analysis, comparatively rare for non-linear optical spectroscopy, canbe carried out to yield quantitative results.Therefore, our objective in the present thesis is to develop an experimentalapproach based on infrared spectroscopy for the characterization of the complexinfrared dielectric function of amorphous thin films grown on a substrate, whichis inaccessible by other means. The proposed approach is based on the analysis ofthe infrared reflectivity spectrum of the considered film/substrate using a numericaltechnique combining the Fresnel theory and the Kramers-Kronig conversiontheorem.We used the technique developed to deduce the complex infrared dielectricfunction of amorphous silicon carbide thin films deposited on silicon at differenttemperatures and pressure levels using the pulsed laser deposition (PLD) growthtechnique. The results obtained showed that the growth temperature does nothave a significant effect on the dielectric properties of the amorphous films. However,the variation in pressure allows a substantial modification of the real andimaginary parts of the infrared complex dielectric function of the amorphoussilicon carbide film.We believe that the optical technique developed in this work constitutes anon-destructive method for the characterization of relevant infrared properties ofamorphous materials, which so far are not clear to materials scientists.
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- رقم الوثيقة
- 0054afab-619e-4b6b-a462-8d84d18f9d96
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- صيغة المصدر
- رسائل ماجيستير
- نوع الملف
- pdf text
- أسماء الملفات
- 2026075_1.pdf
بيانات النشر
- ألقاب المؤلفين
- [{"name_ar":"Marwa Youssef Dakik","title_ar":"اعداد","title_en":"Preparation"},{"name_ar":"Michel Kazan","title_ar":"اشراف","title_en":"Supervision"}]
- اللغة
- English
المصدر والدورية
- اسم المصدر
- Method for Deriving the Complex Infrared Dielectric Function of Amorphous Thin Films from Infrared Reflectivity Spectroscopy
المحتوى والصفحات
- عدد الصفحات
- 0
- كلمات الباحثين
- Show simple item record dc.contributor.advisor Kazan, Michel dc.contributor.author Dakik, Marwa dc.date.accessioned 2020-09-23T18:02:08Z dc.date.available 2020-09-23T18:02:08Z dc.date.issued 2020-09-23 dc.identifier.uri http://hdl.handle.net/10938/22116 dc.description Prof. Malek TabbalDr. Sara Najem dc.description.abstract Although advanced nonlinear optical techniques have demonstrated high potentialfor examining elementary excitations in semiconductors, infrared reflectivityanalysis remains the most quantitative technique because simple theories canbe used to describe the material response to an infrared wavelength excitation.Line shape analysis, comparatively rare for non-linear optical spectroscopy, canbe carried out to yield quantitative results.Therefore, our objective in the present thesis is to develop an experimentalapproach based on infrared spectroscopy for the characterization of the complexinfrared dielectric function of amorphous thin films grown on a substrate, whichis inaccessible by other means. The proposed approach is based on the analysis ofthe infrared reflectivity spectrum of the considered film/substrate using a numericaltechnique combining the Fresnel theory and the Kramers-Kronig conversiontheorem.We used the technique developed to deduce the complex infrared dielectricfunction of amorphous silicon carbide thin films deposited on silicon at differenttemperatures and pressure levels using the pulsed laser deposition (PLD) growthtechnique. The results obtained showed that the growth temperature does nothave a significant effect on the dielectric properties of the amorphous films. However,the variation in pressure allows a substantial modification of the real andimaginary parts of the infrared complex dielectric function of the amorphoussilicon carbide film.We believe that the optical technique developed in this work constitutes anon-destructive method for the characterization of relevant infrared properties ofamorphous materials, which so far are not clear to materials scientists. dc.language.iso en
إشراف وإعداد
- الإشراف
- Michel Kazan
- الإعداد
- Marwa Youssef Dakik
الاقتباسات الببليوغرافية
APA
MLA